If your exclude a group or remove the assignment, Intune doesn't remove the settings configured earlier by the polices. They stay on. To remove the settings, you will have to create another set of policy with desired configuration(revert in your case) and deploy that to the intended group of devices\users. The same group should either be added to the exclusions of existing policy containing the settings that you want to remove or the assignment itself will need to be removed. This is needed to avoid conflicts.
Intune Configuration Profile Remove
If I have a configuration profile with some administrative template settings set and assigned to a group. To remove those settings would I just move that group to the Excluded group? Or would I need to modify the settings in that config profile and then keep that group in the Included groups? Or would just removing the groups from that configuration profile set all of those settings back to their defaults?
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Brownmattc 6 Reputation points
2022-11-08T21:38:25.26+00:00 Windows devices: After you remove or unassign the profile, have the Azure AD user sign in to the device, and sync with the Intune service.
Intune settings are based on the Windows configuration service provider (CSPs). The behavior depends on the CSP. Some CSPs remove the setting, and some CSPs keep the setting, also called tattooing.
Source: https://learn.microsoft.com/en-us/mem/intune/configuration/device-profile-troubleshoot