Hi @Steve Roman,
Is this Office 2021 a retail version that you bound the key with your Microsoft account, and then log in to the activate Office?
If so, please sign out your account from Office apps, and sign back for a check.
Besides, you may uninstall Office via tool, then restart your machine, reinstall it from Subscriptions & Services page. Or following the article: Download, install, or reinstall Microsoft 365, Office 2024, or Office 2021 on a PC or Mac.